ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces
5 years ago

Novel Perovskite Solar Cell Architecture Featuring Efficient Light Capture and Ultrafast Carrier Extraction

Novel Perovskite Solar Cell Architecture Featuring Efficient Light Capture and Ultrafast Carrier Extraction
Yan Liu, Junjie Xie, Lei Lei, Sheng Zhang, Qipeng Cao, Bangjiao Ye, Jun Shao, Xiaojie Ni, Songwang Yang, Yu Yu
A new perovskite solar cell (PSC) structure with a functionalized interface between perovskite and a hole transport material has been proposed in this report. The short circuit current density of PSC was notably enhanced with the novel architecture (with an increase of 8.7%), and a power conversion efficiency (PCE) of 16.93% was achieved. With the increased perovskite/hole conductor interface, hysteresis suppression was observed. The advantages of this structure in light-harvesting efficiency, trap density, and carrier separation rate were proved by various characterization and analysis studies. It is noteworthy that a PCE of 14.67% was achieved with poly(3-hexyl-thiophene), which to our knowledge is the highest performing PSC based on this material.

Publisher URL: http://dx.doi.org/10.1021/acsami.7b03666

DOI: 10.1021/acsami.7b03666

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