3 years ago

Experimental validation of a nuclear forensics methodology for source reactor-type discrimination of chemically separated plutonium

Jeremy M. Osborn, Kevin J. Glennon, Evans D. Kitcher, Jonathan D. Burns, Charles M. Folden, Sunil S. Chirayath

Publication date: Available online 10 November 2018

Source: Nuclear Engineering and Technology

Author(s): Jeremy M. Osborn, Kevin J. Glennon, Evans D. Kitcher, Jonathan D. Burns, Charles M. Folden, Sunil S. Chirayath

Abstract

An experimental validation of a nuclear forensics methodology for the source reactor-type discrimination of separated weapons-useable plutonium is presented. The methodology uses measured values of intra-element isotope ratios of plutonium and fission product contaminants. MCNP radiation transport codes were used for various reactor core modeling and fuel burnup simulations. A reactor-dependent library of intra-element isotope ratio values as a function of burnup and time since irradiation was created from the simulation results. The experimental validation of the methodology was achieved by performing two low-burnup experimental irradiations, resulting in distinct fuel samples containing sub-milligram quantities of weapons-useable plutonium. The irradiated samples were subjected to gamma and mass spectrometry to measure several intra-element isotope ratios. For each reactor in the library, a maximum likelihood calculation was utilized to compare the measured and simulated intra-element isotope ratio values, producing a likelihood value which is proportional to the probability of observing the measured ratio values, given a particular reactor in the library. The measured intra-element isotope ratio values of both irradiated samples and its comparison with the simulation predictions using maximum likelihood analyses are presented. The analyses validate the nuclear forensics methodology developed.

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