Inorganic Chemistry
Inorganic Chemistry
5 years ago

Electric Field Generation and Control of Bipartite Quantum Entanglement between Electronic Spins in Mixed Valence Polyoxovanadate [GeV14O40]8–

Electric Field Generation and Control of Bipartite Quantum Entanglement between Electronic Spins in Mixed Valence Polyoxovanadate [GeV14O40]8–
Andrew Palii, Juan José Borràs-Almenar, Eugenio Coronado, Juan Modesto Clemente-Juan, Boris Tsukerblat, Sergey Aldoshin, Salvador Cardona-Serra
We show that an external homogeneous electric field can be used as a tool to create a controllable quantum entanglement between the two weakly coupled electronic spins of the mixed valence polyoxoanion [GeV14O40]8−. Within a simplified two-level picture of the electronic pair based on ab initio analysis of the parameters, we evaluate the temperature and field dependencies of concurrence and thus indicate that the entanglement can be controlled via the temperature, magnitude, and orientation of the electric field with respect to molecular axes.

Publisher URL: http://dx.doi.org/10.1021/acs.inorgchem.7b00991

DOI: 10.1021/acs.inorgchem.7b00991

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