3 years ago

Light-responsive organic flashing electron ratchet [Chemistry]

Light-responsive organic flashing electron ratchet [Chemistry]
Ofer Kedem, Mark A. Ratner, Bryan Lau, Emily A. Weiss

Ratchets are nonequilibrium devices that produce directional motion of particles from nondirectional forces without using a bias, and are responsible for many types of biological transport, which occur with high yield despite strongly damped and noisy environments. Ratchets operate by breaking time-reversal and spatial symmetries in the direction of transport through application of a time-dependent potential with repeating, asymmetric features. This work demonstrates the ratcheting of electrons within a highly scattering organic bulk-heterojunction layer, and within a device architecture that enables the application of arbitrarily shaped oscillating electric potentials. Light is used to modulate the carrier density, which modifies the current with a nonmonotonic response predicted by theory. This system is driven with a single unbiased sine wave source, enabling the future use of natural oscillation sources such as electromagnetic radiation.

Publisher URL: http://www.pnas.org/content/114/33/8698.short

DOI: 10.1073/pnas.1705973114

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