3 years ago

Iridium(III)-Catalyzed Synthesis of Benzimidazoles via C–H Activation and Amidation of Aniline Derivatives

Iridium(III)-Catalyzed Synthesis of Benzimidazoles via C–H Activation and Amidation of Aniline Derivatives
Yunyun Li, Xifa Yang, Xingwei Li, Jintao Xia
Ir(III)-catalyzed synthesis of benzimidazoles has been realized under redox-neutral conditions by annulation of aniline derivatives with dioxazolones. The reaction proceeded via a C–H activation–amidation–cyclization pathway with a decent substrate scope.

Publisher URL: http://dx.doi.org/10.1021/acs.orglett.7b01356

DOI: 10.1021/acs.orglett.7b01356

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