5 years ago

[FeFe] Hydrogenase active site model chemistry in a UiO-66 metal-organic framework

[FeFe] Hydrogenase active site model chemistry in a UiO-66 metal-organic framework
Souvik Roy, Sascha Ott, Sonja Pullen
CO[rightward arrow]phosphine ligand exchange reactions on [FeFe(dcbdt)(CO)6] incorporated in UiO-66(Zr) afford selectively the disubstituted UiO-66-[FeFe(dcbdt)(CO)4(PX3)2] which can be protonated quantitatively to afford the bridging hydride UiO-66-[FeFe(dcbdt)([small mu ]-H)(CO)4(PX3)2].

Publisher URL: http://feeds.rsc.org/~r/rss/CC/~3/nuRLV6lRgsQ/C7CC01620D

DOI: 2017/CC/C7CC01620D

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