Accounts of Chemical Research
Accounts of Chemical Research
5 years ago

Novel in Situ Techniques for Studies of Model Catalysts

Novel in Situ Techniques for Studies of Model Catalysts
Chu Zhang, Jianfeng Zhou, Mikhail Shipilin, Uta Hejral, Lindsay R. Merte, Johan Zetterberg, Sara Blomberg, Edvin Lundgren, Johan Gustafson
Motivated mainly by catalysis, gas–surface interaction between single crystal surfaces and molecules has been studied for decades. Most of these studies have been performed in well-controlled environments and have been instrumental for the present day understanding of catalysis, providing information on surface structures, adsorption sites, and adsorption and desorption energies relevant for catalysis. However, the approach has been criticized for being too far from a catalyst operating under industrial conditions at high temperatures and pressures. To this end, a significant amount of effort over the years has been used to develop methods to investigate catalysts at more realistic conditions under operating conditions. One result from this effort is a vivid and sometimes heated discussion concerning the active phase for the seemingly simple CO oxidation reaction over the Pt-group metals in the literature.

Publisher URL: http://dx.doi.org/10.1021/acs.accounts.7b00281

DOI: 10.1021/acs.accounts.7b00281

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