4 years ago

Network Dimensionality of Selected Uranyl(VI) Coordination Polymers and Octopus-like Uranium(IV) Clusters

Network Dimensionality of Selected Uranyl(VI) Coordination Polymers and Octopus-like Uranium(IV) Clusters
Aaron M. Tondreau, Marisa J. Monreal, James M. Boncella, Henry S. La Pierre, Stosh A. Kozimor, Brian L. Scott, Ralph A. Zehnder, Justin N. Cross, Matthias Zeller
We present the synthesis of various uranium open frameworks utilizing slow diffusion methods at room temperature. The structural properties and topologies of these materials are described, and we illustrate that the glutarate linker assists in obtaining three-dimensional networks, while the rather rigid terephthalate derivatives restrict the connectivity of the uranyl unit to form one-dimensional and two-dimensional underlying network systems.

Publisher URL: http://dx.doi.org/10.1021/acs.cgd.7b01165

DOI: 10.1021/acs.cgd.7b01165

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