ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces
5 years ago

Enhancing Mechanical and Thermal Properties of Epoxy Nanocomposites via Alignment of Magnetized SiC Whiskers

Enhancing Mechanical and Thermal Properties of Epoxy Nanocomposites via Alignment of Magnetized SiC Whiskers
Konstantin G. Kornev, James Townsend, Pavel Aprelev, Ruslan Burtovyy, Igor Luzinov
This research is focused on the fabrication and properties of epoxy nanocomposites containing magnetized SiC whiskers (MSiCWs). To this end, we report an original strategy for fabrication of magnetically active SiCWs by decorating the whiskers with magnetic (iron oxide) nanoparticles via polymer–polymer (poly(acrylic acid)/poly(2-vinyl pyridine)) complexation. The obtained whiskers demonstrated a substantial magnetic response in the polymerizing epoxy resin, with application of only a 20 mT (200 G) magnetic field. We also found that the whiskers chemically reacted with the epoxy resin, causing formation of an extended interphase near the boundary of the whiskers. The SiC whiskers oriented with the magnetic field demonstrated positive effects on the behavior of epoxy-based nanocomposites. Namely, the aligned MSiCWs enhanced the thermomechanical properties of the materials significantly above that of the neat epoxy and epoxy nanocomposite, with randomly oriented whiskers.

Publisher URL: http://dx.doi.org/10.1021/acsami.7b04546

DOI: 10.1021/acsami.7b04546

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